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Journal Articles

Anomalous behavior of liquid molecules near solid nanoparticles; Novel interpretation on thermal conductivity enhancement in nanofluids

Hashimoto, Shunsuke*; Yamaguchi, Satoshi*; Harada, Masashi*; Nakajima, Kenji; Kikuchi, Tatsuya*; Oishi, Kazuki*

Journal of Colloid and Interface Science, 638, p.475 - 486, 2023/05

https://doi.org/10.1016/j.jcis.2023.01.101

Times Cited Count：2 Percentile：66.51(Chemistry, Physical)

Recently, it has been reported that anomalous improvement in the thermal conductivity of nanofluid composed of base liquids and dispersed solid nanoparticles, compared to the theoretically predicted value calculated from the particle fraction. Generally, the thermal conductivity values of gases and liquids are dominated by the mean free path of the molecules during translational motion. Herein, we present solid evidence showing the possible contribution of the vibrational behavior of liquid molecules around nanoparticles to increasing these thermal conductivities.

Journal Articles

Spin gap in the weakly interacting quantum spin chain antiferromagnet KCuPO $_{4}$ H $_{2}$ O

Fujihara, Masayoshi; Hagihara, Masato; Morita, Katsuhiro*; Murai, Naoki; Koda, Akihiro*; Okabe, Hirotaka*; Mitsuda, Setsuo*

Physical Review B, 107(5), p.054435_1 - 054435_8, 2023/02

https://doi.org/10.1103/PhysRevB.107.054435

Times Cited Count：0 Percentile：0(Materials Science, Multidisciplinary)

The = 1/2 Heisenberg linear chain antiferromagnet is the simplest spin model; nevertheless it serves as a platform for various quantum many-body phenomena. Here, we report the magnetic behavior of a quasi-one-dimensional antiferromagnet KCuPO $_{4}$ H $_{2}$ O. A long-range commensurate antiferromagnetic order with ordered moment 0.31(1) $mu_{rm{B}}$ per spin occurs at $T_{rm{N}}$ = 11.7(1) K. Above $T_{rm{N}}$ , the inelastic neutron excitation is characterized by a two spinon continuum. The intrachain interaction and interchain interaction are estimated to be 172 K and 4.25(4) K, respectively; thus the ratio of the / = 0.0247(3). At lower energies, below $T_{rm{N}}$ , a spin gap is observed in the dispersive excitations. These results are consistent with characteristics observed in weakly interacting = 1/2 Heisenberg chain system.

Journal Articles

Hyperfine splitting and nuclear spin polarization in NdPdAl and NdPd $_{20}$ Ge

Metoki, Naoto; Shibata, Kaoru; Matsuura, Masato*; Kitazawa, Hideaki*; Suzuki, Hiroyuki*; Yamauchi, Hiroki; Hagihara, Masato; Frontzek, M. D.*; Matsuda, Masaaki*

Journal of the Physical Society of Japan, 91(5), p.054710_1 - 054710_6, 2022/05

https://doi.org/10.7566/JPSJ.91.054710

Times Cited Count：0 Percentile：0(Physics, Multidisciplinary)

Hyperfine splitting of Nd nuclei in NdPdAl has been studied by means of high-resolution neutron spectroscopy. We observed inelastic peaks at eV coming from the hyperfine splitting in the magnetically ordered phase due to the hyperfine interactions between Nd nuclei (=7/2) and the 4 electrons with ground state composed of mainly . At very low temperatures, nuclear spin of Nd is polarized with increasing occupation probability of low energy levels and contributes to the enhancement of the antiferromagnetic Bragg intensities: the elastic non-spin-flip channel is dominant. As an application of this phenomenon, we determined the Nd moment and hyperfine splitting from the temperature dependence of an antiferromagnetic Bragg intensities for NdPd $_{20}$ Ge.

Journal Articles

Mictomagnetism and suppressed thermal conduction of the prototype high-entropy alloy CrMnFeCoNi

Yang, J.*; Ren, W.*; Zhao, X.*; Kikuchi, Tatsuya*; Miao, P.*; Nakajima, Kenji; Li, B.*; Zhang, Z.*

Journal of Materials Science & Technology, 99, p.55 - 60, 2022/02

https://doi.org/10.1016/j.jmst.2021.04.077

Times Cited Count：5 Percentile：41.35(Materials Science, Multidisciplinary)

High-entropy alloys are characteristic of extensive atomic occupational disorder on high-symmetric lattices, differing from traditional alloys. Here, we investigate magnetic and thermal transport properties of the prototype face-centered-cubic high-entropy alloy CrMnFeCoNi by combining physical properties measurements and neutron scattering. Direct-current (dc) and alternating-current (ac) magnetizations measurements indicate a mictomagnetic behavior with coexisting antiferromagnetic and ferromagnetic interactions in the entire temperature region and three anomalies are found at about 80, 50, and 20 K, which are related to the paramagnetic to antiferromagnetic transition, the antiferromagnetic to ferromagnetic transition, and the spin freezing, respectively. The electrical and thermal conductivities are significantly reduced compared to Ni and the temperature dependence of lattice thermal conductivity exhibits a glass-like plateau. Inelastic neutron scattering measurements suggest weak anharmonicity so that the thermal transport is expected to be dominated by the defect scattering.

Journal Articles

Nanometric fluctuations of sound velocity in alkali borate glasses and fragility of respective melts

Kojima, Seiji*; Novikov, V. N.*; Kofu, Maiko; Yamamuro, Osamu*

Physica Status Solidi (B), 257(11), p.200073_1 - 200073_6, 2020/11

https://doi.org/10.1002/pssb.202000073

Times Cited Count：3 Percentile：19.68(Physics, Condensed Matter)

Journal Articles

-electron states of NpPdAl and the isostructural family; Heavy fermion superconductivity accompanied by valence crossover

Metoki, Naoto

Kotai Butsuri, 55(7), p.285 - 296, 2020/07

Electron states are the main theme of "solid-state physics", which is essential for microscopic understanding of multipoles and superconductivity, etc. Rare earths (4) and actinides (5) provide variety of interesting states realized with competing interactions between the increasing number of electrons. Since crystal field splitting of many-body electron system is smaller than the bandwidth, (1) high resolution experiments are needed, (2) essentially no clear spectrum with well defined peaks is expected in itinerant Ce and U compounds, and (3) Np and Pu is strictly regulated. Therefore, systematic research on magnetic excitations by neutron scattering experiments of localized compounds and rare earth iso-structural reference is useful. We describe the electron states of heavy electron compounds NpPdAl and actinide and rare earth based iso-structural family.

Journal Articles

Gapless spin liquid in a square-kagome lattice antiferromagnet

Fujihara, Masayoshi*; Morita, Katsuhiro*; Mole, R.*; Mitsuda, Setsuo*; Toyama, Takami*; Yano, Shinichiro*; Yu, D.*; Sota, Shigetoshi*; Kuwai, Tomohiko*; Koda, Akihiro*; et al.

Nature Communications (Internet), 11, p.3429_1 - 3429_7, 2020/07

https://doi.org/10.1038/s41467-020-17235-z

Times Cited Count：37 Percentile：90.63(Multidisciplinary Sciences)

Journal Articles

Multiple magnetic bilayers and unconventional criticality without frustration in BaCuSiO

Allenspach, S.*; Biffin, A.*; Stuhr, U.*; Tucker, G. S.*; Kawamura, Seiko; Kofu, Maiko; Voneshen, D. J.*; Boehm, M.*; Normand, B.*; Laflorencie, N.*; et al.

Physical Review Letters, 124(17), p.177205_1 - 177205_7, 2020/05

https://doi.org/10.1103/PhysRevLett.124.177205

Times Cited Count：10 Percentile：65.11(Physics, Multidisciplinary)

Journal Articles

Neutron scattering studies of static and dynamic correlation lengths in alkali metal borate glasses

Kojima, Seiji*; Novikov, V. N.*; Kofu, Maiko; Yamamuro, Osamu*

Journal of Non-Crystalline Solids, 518, p.18 - 23, 2019/08

https://doi.org/10.1016/j.jnoncrysol.2019.05.005

Times Cited Count：6 Percentile：29.81(Materials Science, Ceramics)

Journal Articles

Continuum excitation and pseudospin wave in quantum spin-liquid and quadrupole ordered states of Tb $_{2+x}$ Ti $_{2-x}$ O $_{7+y}$

Kadowaki, Hiroaki*; Wakita, Mika*; Fk, B.*; Ollivier, J.*; Kawamura, Seiko; Nakajima, Kenji; Takatsu, Hiroshi*; Tamai, Mototake*

Journal of the Physical Society of Japan, 87(6), p.064704_1 - 064704_6, 2018/06

https://doi.org/10.7566/JPSJ.87.064704

Times Cited Count：9 Percentile：57.38(Physics, Multidisciplinary)

The ground states of the frustrated pyrochlore oxide Tb $_{2+x}$ Ti $_{2-x}$ O $_{7+y}$ have been studied by inelastic neutron scattering experiments. Three single-crystal samples are investigated; one shows no phase transition ( $x = -0.007 < x_{c} < sim -0.0025$ ), being a putative quantum spin-liquid (QSL), and the other two () show electric quadrupole ordering (QO) below $T_{c} sim 0.5$ K. The QSL sample shows continuum excitation spectra with an energy scale 0.1 meV as well as energy-resolution-limited (nominally) elastic scattering. As is increased, pseudospin wave of the QO state emerges from this continuum excitation, which agrees with that of powder samples and consequently verifies good control for the present single crystal samples.

Journal Articles

Effect of rattling motion without cage structure on lattice thermal conductivity in LaOBiS $_{2-x}$ Se

Lee, C. H.*; Nishida, Atsuhiro*; Hasegawa, Takumi*; Nishiate, Hirotaka*; Kunioka, Haruno*; Kawamura, Seiko; Nakamura, Mitsutaka; Nakajima, Kenji; Mizuguchi, Yoshikazu*

Applied Physics Letters, 112(2), p.023903_1 - 023903_4, 2018/01

https://doi.org/10.1063/1.5010373

Times Cited Count：28 Percentile：77.9(Physics, Applied)

Low energy phonons in LaOBiS $_{2-x}$ Se are studied using inelastic neutron scattering. Dispersionless flat phonon branches that are mainly associated with a large vibration of Bi atoms are observed at a relatively low energy of = 6 - 6.7 meV. The phonon energy softens upon Se doping owing to its heavier atomic mass than S atom and the expansion of lattice constant. Simultaneously, the lattice thermal conductivity lowered upon Se doping as the same manner of the phonon softening. These suggest that despite the lack of an oversized cage in LaOBiS $_{2-x}$ Se, rattling motions of Bi atoms can scatter phonon like rattling in cage compounds, contributing to enhance the thermoelectric property.

Journal Articles

Vibrational states of atomic hydrogen in bulk and nanocrystalline palladium studied by neutron spectroscopy

Kofu, Maiko; Hashimoto, Naoki*; Akiba, Hiroshi*; Kobayashi, Hirokazu*; Kitagawa, Hiroshi*; Iida, Kazuki*; Nakamura, Mitsutaka; Yamamuro, Osamu*

Physical Review B, 96(5), p.054304_1 - 054304_7, 2017/08

https://doi.org/10.1103/PhysRevB.96.054304

Times Cited Count：15 Percentile：58.3(Materials Science, Multidisciplinary)

The vibrational states of hydrogen atoms in bulk and nanocrystalline palladium were examined in a wide energy region meV using neutron spectroscopy. In bulk PdH $_{0.73}$ , the vibrational excitations of H atoms were roughly reproduced by the quantum harmonic oscillator (QHO) model. In PdH $_{0.42}$ nanocrystals with a diameter of 8 nm, however, additional vibrational excitations were found at energies above 80 meV. The energies and intensities of the additional states were not explained by QHO but reasonably described as vibrations in a highly anharmonic trumpet-like potential. The additional excitations are attributed to the vibrations of H atoms at tetrahedral sites in the subsurface region stabilized by surface effects. This is an experimental work which clearly detects hydrogen vibration metal nanoparticles.